{"id":18139,"date":"2018-03-07T06:08:03","date_gmt":"2018-03-06T22:08:03","guid":{"rendered":"\/\/www.gsbet888.com\/?p=18139"},"modified":"2019-08-02T18:51:54","modified_gmt":"2019-08-02T10:51:54","slug":"cathleen-m-crudden","status":"publish","type":"post","link":"\/\/www.gsbet888.com\/chemists\/2018\/03\/cathleen-m-crudden.html","title":{"rendered":"Cathleen M. Crudden"},"content":{"rendered":"<p>Cathleen M. Crudden\u30011967\u5e7411\u670823\u65e5\u2013 \u52a0\u62ff\u5927\u7684\u6709\u673a\u5316\u5b66\u5bb6\u3002Queen&#8217;s \u5927\u5b66\u6559\u6388(\u7167\u7247:\u5f15\u7528\u81eaQueen\u2019s\u5927\u5b66\u5316\u5b66\u79d1HP)<\/p>\n<h4>\u7ecf\u5386<\/h4>\n<p>1989 \u591a\u4f26\u591a\u5927\u5b66\u3000\u6bd5\u4e1a (M. Lautens \u6559\u6388)<br \/>\n1990 \u591a\u4f26\u591a\u5927\u5b66\u3000\u7855\u58eb\u5b66\u4f4d (M. Lautens \u6559\u6388)<br \/>\n1995 \u6e25\u592a\u534e\u5927\u5b66\u3000\u535a\u58eb\u5b66\u4f4d (H. Alper\u6559\u6388)<br \/>\n1995-1996 \u4f0a\u5229\u8bfa\u4f0a\u5927\u5b66\u9999\u69df\u5206\u6821\u3000\u535a\u58eb\u540e\u7814\u7a76\u5458 (Scott. E. Denmark\u6559\u6388)<br \/>\n1996-2000 \u65b0\u4e0d\u4f26\u745e\u514b\u5927\u5b66\u3000\u52a9\u6559<br \/>\n2000-2001 \u65b0\u4e0d\u4f26\u745e\u514b\u5927\u5b66\u3000\u526f\u6559\u6388<br \/>\n2001-2002 \u65b0\u4e0d\u4f26\u745e\u514b\u5927\u5b66\u3000\u6559\u6388<br \/>\n2002-2007 Queen&#8217;s \u5927\u5b66\u3000\u526f\u6559\u6388 (Queen\u2019s National Scholar)<br \/>\n2009- \u30af\u30a4\u30fc\u30f3\u30ba\u5927\u5b66\u3000\u6559\u6388<br \/>\n2013- \u540d\u53e4\u5c4b\u5927\u5b66\u3000Transformative\u751f\u547d\u5206\u5b50\u7814\u7a76\u6240(ITbM)\u3000\u5ba2\u5ea7\u6559\u6388\u3001\u6d77\u5916\u4e3b\u4efb\u7814\u7a76\u8005<\/p>\n<p>\u517c\u4efb<\/p>\n<p>2011 \u52a0\u62ff\u5927\u5316\u5b66\u4f1a\u3000\u526f\u4f1a\u957f<br \/>\n2012 \u52a0\u62ff\u5927\u5316\u5b66\u4f1a\u3000\u4f1a\u957f<\/p>\n<h4>\u83b7\u5956\u7ecf\u5386<\/h4>\n<p>2010 NSERC Accelerator Awarde<br \/>\n2010 Catalysis Society Lectureship Award<br \/>\n2011 Clara Benson Award<br \/>\n2012-2013 President, Canadian Society of Chemistry<br \/>\n2014 Fellow, Chemical Institute of Canada<br \/>\n2014-2018 Scientific Council Member, The Sainsbury Lab., UK<br \/>\n2015-2016 Killam Research Fellow<br \/>\n2017 R. U. Lemieux Award, Canadian Society for Chemistry<br \/>\n2017 SYNLETT Best Paper Award 2017<br \/>\n2018 Catalysis Award, Chemical Institution of Canada<\/p>\n<h4>\u7814\u7a76\u6982\u8981<\/h4>\n<p><strong><u>\u5229\u7528\u6709\u673a\u787c\u5316\u5408\u7269\u8fdb\u884c\u4e0d\u5bf9\u79f0\u50ac\u5316\u53cd\u5e94\u7684\u7814\u7a76\u8fdb\u5c55<\/u><\/strong><\/p>\n<p>\u9ad8\u6548\u73af\u5883\u8d1f\u8377\u5c0f\u7684\u787c\u5316\u5b66\u4e3a\u7acb\u8db3\u70b9\u8fdb\u884c\u53cd\u5e94\u5f00\u53d1\u3002\u5176\u4e2d\u4ee3\u8868\u4f8b\u6709\u3001\u4f7f\u7528\u624b\u6027\u4ef2\u787c\u9178\u916f\u7684Suzuki-Miyaura\u4ea4\u53c9\u5076\u8054\u53cd\u5e94[1]\u3002\u540c\u65f6\uff0c\u901a\u8fc7\u4f7f\u7528\u72ec\u81ea\u5f00\u53d1\u7684\u781c\u7c7b\u5316\u5408\u7269\u8fdb\u884cC-H\u82b3\u57fa\u5316\u53cd\u5e94\u7b49\u5076\u8054\u53cd\u5e94\uff0c\u7528\u4e8e\u9ad8\u6548\u5408\u6210\u4e09\u82b3\u57fa\u7532\u70f7[2]\u548c\u56db\u82b3\u57fa\u7532\u70f7[3]\uff0c\u5b83\u4eec\u662f\u836f\u7269\u548c\u989c\u6599\u4e2d\u7684\u6709\u7528\u9aa8\u67b6\u3002<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter wp-image-18141 size-full\" src=\"https:\/\/assets.www.gsbet888.com\/uploads\/2018\/03\/2018-02-25_17-27-56.png\" alt=\"\" width=\"735\" height=\"334\" srcset=\"https:\/\/assets.www.gsbet888.com\/uploads\/2018\/03\/2018-02-25_17-27-56.png 735w, https:\/\/assets.www.gsbet888.com\/uploads\/2018\/03\/2018-02-25_17-27-56-300x136.png 300w, https:\/\/assets.www.gsbet888.com\/uploads\/2018\/03\/2018-02-25_17-27-56-680x309.png 680w\" sizes=\"(max-width: 735px) 100vw, 735px\" \/><\/p>\n<p><strong><u>\u624b\u6027\u4ecb\u5b54\u6750\u6599\u7684\u7814\u5236<\/u><\/strong><\/p>\n<p>\u901a\u8fc7\u4f7f\u7528\u4e0d\u5bf9\u79f0\u5355\u4f53\u4f5c\u4e3a\u624b\u6027\u63ba\u6742\u5242\uff0c\u6210\u529f\u5728\u4e16\u754c\u4e0a\u9996\u6b21\u5f00\u53d1\u624b\u6027\u4ecb\u5b54\u4e8c\u6c27\u5316\u7845<sup>[4]<\/sup>\u3002\u529f\u80fd\u5316\u7684\u624b\u6027\u4ecb\u5b54\u4e8c\u6c27\u5316\u7845\u53ef\u4ee5\u643a\u5e26\u91d1\u5c5e\u3002\u901a\u8fc7\u8fd9\u79cd\u6027\u8d28\u53ef\u4ee5\u7528\u4f5c\u53cd\u5e94\u540e\u91d1\u5c5e\u6e05\u9664\u5242\u4f7f\u5f97\u50ac\u5316\u5242\u53ef\u4ee5\u5faa\u73af\u5229\u7528\uff0c\u6709\u5e0c\u671b\u5b9e\u73b0\u5de5\u4e1a\u5316\u3002<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter wp-image-18142 size-full\" src=\"https:\/\/assets.www.gsbet888.com\/uploads\/2018\/03\/2018-02-25_17-28-21.png\" alt=\"\" width=\"929\" height=\"197\" srcset=\"https:\/\/assets.www.gsbet888.com\/uploads\/2018\/03\/2018-02-25_17-28-21.png 929w, https:\/\/assets.www.gsbet888.com\/uploads\/2018\/03\/2018-02-25_17-28-21-300x64.png 300w, https:\/\/assets.www.gsbet888.com\/uploads\/2018\/03\/2018-02-25_17-28-21-768x163.png 768w, https:\/\/assets.www.gsbet888.com\/uploads\/2018\/03\/2018-02-25_17-28-21-680x144.png 680w\" sizes=\"(max-width: 929px) 100vw, 929px\" \/><\/p>\n<p><strong><em><u>N-<\/u><\/em><u>\u6742\u73af\u5361\u5bbe\u914d\u5408\u7269\u50ac\u5316\u53cd\u5e94\u7684\u7814\u7a76\u8fdb\u5c55<\/u><\/strong><\/p>\n<p>\u6211\u4eec\u5df2\u7ecf\u5f00\u53d1\u4e86\u5404\u79cdRh &#8211; NHC\u914d\u5408\u7269\uff0c\u5e76\u4f7f\u7528\u5b83\u4eec\u5f00\u53d1\u62a5\u9053\u4e86\u52a0\u6c22\u7532\u9170\u5316\u548cC &#8211; H\u787c\u5316\u53cd\u5e94<sup>[5]<\/sup>\u3002\u53e6\u5916\uff0c\u6210\u529f\u901a\u8fc7\u6c27\u4e0eRh-NHC\u7edc\u5408\u7269\u53cd\u5e94\u6765\u5206\u79bb\u914d\u4f4d\u6709\u6c27\u5206\u5b50\u800c\u4e0d\u5f15\u8d77\u6c27\u5316\u7684\u7edc\u5408\u7269<sup>[6]<\/sup>\u3002<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter wp-image-18143 size-full\" src=\"https:\/\/assets.www.gsbet888.com\/uploads\/2018\/03\/2018-02-25_17-29-54.png\" alt=\"\" width=\"708\" height=\"352\" srcset=\"https:\/\/assets.www.gsbet888.com\/uploads\/2018\/03\/2018-02-25_17-29-54.png 708w, https:\/\/assets.www.gsbet888.com\/uploads\/2018\/03\/2018-02-25_17-29-54-300x149.png 300w, https:\/\/assets.www.gsbet888.com\/uploads\/2018\/03\/2018-02-25_17-29-54-680x338.png 680w\" sizes=\"(max-width: 708px) 100vw, 708px\" \/><\/p>\n<p>\u8fd1\u5e74\u6765\uff0c\u8bfe\u9898\u7ec4\u5f00\u53d1\u4f7f\u7528\u75311,2,3-\u4e09\u5511\u9393\u76d0\u548c\u787c\u70f7\u5236\u5907\u7684Mesoionic borenium\u50ac\u5316\u53cd\u5e94<sup>[7]<\/sup>\u3002Mesoionic borenium\u50ac\u5316\u5242\u4f5c\u4e3aFLP(frustrated Lewis pair)\u8fdb\u884c\u4f5c\u7528\u3002<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter wp-image-18144 size-full\" src=\"https:\/\/assets.www.gsbet888.com\/uploads\/2018\/03\/2018-02-25_17-30-15.png\" alt=\"\" width=\"591\" height=\"181\" srcset=\"https:\/\/assets.www.gsbet888.com\/uploads\/2018\/03\/2018-02-25_17-30-15.png 591w, https:\/\/assets.www.gsbet888.com\/uploads\/2018\/03\/2018-02-25_17-30-15-300x92.png 300w\" sizes=\"(max-width: 591px) 100vw, 591px\" \/><\/p>\n<p><strong><u>\u4f7f\u7528NHC\u914d\u4f53\u7684\u81ea\u7ec4\u88c5\u5355\u5c42<\/u><\/strong><\/p>\n<p>\u6210\u529f\u5730\u7528NHC\u914d\u4f53\u901a\u8fc7\u91d1\u5c5e &#8211; \u78b3\u952e\u5f62\u6210\u81ea\u7ec4\u7ec7\u6765\u4f7f\u91d1\u7684\u5355\u6676\u8868\u9762\u529f\u80fd\u5316<sup>[8]<\/sup>\u3002\u4e0e\u4f20\u7edf\u7684\u5def\u57fa\u5b98\u80fd\u5316\u5355\u5206\u5b50\u5c42\u76f8\u6bd4\uff0c\u5b83\u5bf9\u70ed\uff0c\u9178\uff0c\u78b1\u548c\u6c27\u5316\u5242\u5177\u6709\u5f88\u9ad8\u7684\u8010\u53d7\u6027\u3002<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter wp-image-18145 size-full\" src=\"https:\/\/assets.www.gsbet888.com\/uploads\/2018\/03\/2018-02-25_17-30-50.png\" alt=\"\" width=\"855\" height=\"272\" srcset=\"https:\/\/assets.www.gsbet888.com\/uploads\/2018\/03\/2018-02-25_17-30-50.png 855w, https:\/\/assets.www.gsbet888.com\/uploads\/2018\/03\/2018-02-25_17-30-50-300x95.png 300w, https:\/\/assets.www.gsbet888.com\/uploads\/2018\/03\/2018-02-25_17-30-50-768x244.png 768w, https:\/\/assets.www.gsbet888.com\/uploads\/2018\/03\/2018-02-25_17-30-50-680x216.png 680w\" sizes=\"(max-width: 855px) 100vw, 855px\" \/><\/p>\n<h4>Comment<\/h4>\n<ul>\n<li><\/li>\n<li>\u62c5\u4efb\u8fc7\u4e16\u754c\u6700\u5927\u89c4\u6a21\u7684\u5316\u5b66\u5b66\u4f1aPacifichem\u7684\u7ec4\u7ec7\u59d4\u5458(2010\u5e74)\u4e0e\u52a0\u62ff\u5927\u4ee3\u8868(2015\u5e74)\u3002<\/li>\n<\/ul>\n<h4>\u5173\u8054\u6587\u732e<\/h4>\n<ol>\n<li>Imao, D.; Glasspoole, B. W.; Laberge, V. S.; Crudden, C. M. <em>J.\u00a0Am. Chem. Soc. <\/em><strong>2009<\/strong>, <em>131<\/em>, 5024. DOI: <a href=\"http:\/\/dx.doi.org\/10.1002\/anie.200800153\">10.1002\/anie.200800153<\/a><\/li>\n<li>Nambo, M.; Crudden, C. M. <em>Angew.<\/em>\u00a0<em>Chem., Int. Ed. <\/em><strong>2014<\/strong>, <em>53<\/em>, 742. DOI: <a href=\"http:\/\/dx.doi.org\/10.1002\/anie.201307019\">10.1002\/anie.201307019<\/a><\/li>\n<li>Nambo, M.; Yim, J. C. -H.; Fowler, K. G.; Crudden, C. M. <em>Synlett.<\/em>\u00a0<strong>2017<\/strong>, <em>28<\/em>, 2936. DOI: <a href=\"http:\/\/dx.doi.org\/10.1055\/s-0036-1588563\">10.1055\/s-0036-1588563<\/a><\/li>\n<li>MacQuarrie, S.; Thompson, M. P.; Blanc, A.; Mosey, N. J.; Lemieux, R. P.; Crudden, C. M. <em>J.<\/em>\u00a0<em>Am. Chem. Soc. <\/em><strong>2008<\/strong>, <em>130<\/em>, 14099. DOI: <a href=\"http:\/\/dx.doi.org\/10.1021\/ja804866e\">10.1021\/ja804866e<\/a><\/li>\n<li>[a] Chen, A. C.; Ren, L.; Decken, A.; Crudden, C. M. <em>Organometallics. <\/em><strong>2000<\/strong>, <em>19<\/em>, 3459. DOI: <a href=\"http:\/\/dx.doi.org\/10.1021\/om0003739\">10.1021\/om0003739<\/a> [b] Keske, E. C.; Moore, B. D.; Zenkina, O. V.; Wang, R.; Schatte, G.; Crudden, C. M. <em>Chem. Comm. <\/em><strong>2014<\/strong>, <em>50<\/em>, 9883. DOI: <a href=\"http:\/\/dx.doi.org\/10.1039\/c4cc02499k\">10.1039\/c4cc02499k<\/a><\/li>\n<li>Zenkina, O. V.; Keske, E. C.; Wang, R.; Crudden, C. M. <em>Chem., Int. Ed. <\/em><strong>2011<\/strong>, <em>50<\/em>, 8100. DOI: <a href=\"http:\/\/dx.doi.org\/10.1002\/anie.201103316\">10.1002\/anie.201103316<\/a><\/li>\n<li>Eisenberger, P.; Bestvater, B. P.; Keske, E. C.; Crudden, C. M. <em>Angew.<\/em>\u00a0<em>Chem., Int. Ed. <\/em><strong>2015<\/strong>, <em>54<\/em>, 2467. DOI: <a href=\"http:\/\/dx.doi.org\/10.1002\/anie.201409250\">10.1002\/anie.201409250<\/a><\/li>\n<li>Crudden, C. M.; Horton, J. H.; Ebralidze, I. I.; Zenkina, O. V.; McLean, A. B.; Drevniok, B.; She, Z.; Kraatz, H. -B.; Mosey, N. J.; Seki, T.; Keske, E. C.; Leake, J. D.; Rousina-Webb, A.; Wu, G. <em>Nature.<\/em>\u00a0<em>Chem. <\/em><strong>2014<\/strong>, <em>6<\/em>, 409. DOI: <a href=\"http:\/\/dx.doi.org\/10.1038\/nchem.1891\">10.1038\/nchem.1891<\/a><\/li>\n<\/ol>\n<p>\u672c\u6587\u7248\u6743\u5c5e\u4e8e<strong>\u00a0<a href=\"\/\/www.gsbet888.com\/\">Chem-Station\u5316\u5b66\u7a7a\u95f4<\/a>\uff0c<\/strong> \u6b22\u8fce\u70b9\u51fb\u6309\u94ae\u5206\u4eab\uff0c\u672a\u7ecf\u8bb8\u53ef\uff0c\u8c22\u7edd\u8f6c\u8f7d\uff01 <\/p>\n","protected":false},"excerpt":{"rendered":"Cathleen M. Crudden\u30011967\u5e7411\u670823\u65e5\u2013 \u52a0\u62ff\u5927\u7684\u6709\u673a\u5316\u5b66\u5bb6\u3002Queen&#8217;s \u5927\u5b66\u6559\u6388(\u7167\u7247:\u5f15\u7528\u81eaQueen\u2019s\u5927\u5b66\u5316\u5b66\u79d1HP) \u7ecf\u5386 1989 \u591a\u4f26\u591a\u5927\u5b66\u3000\u6bd5\u4e1a (M. Lautens \u6559\u6388) 1990 \u591a\u4f26\u591a\u5927\u5b66\u3000\u7855\u58eb\u5b66\u4f4d (M. Lautens \u6559\u6388) 1995 \u6e25\u592a\u534e\u5927\u5b66\u3000\u535a\u58eb\u5b66\u4f4d (H. Alper\u6559\u6388) 1995-1996 \u4f0a\u5229\u8bfa\u4f0a\u5927\u5b66\u9999\u69df\u5206\u6821\u3000\u535a\u58eb\u540e\u7814\u7a76\u5458 (Scott. E. Denmark\u6559\u6388) 1996-2000 \u65b0\u4e0d\u4f26\u745e\u514b\u5927\u5b66\u3000\u52a9\u6559 2000-2001 \u65b0\u4e0d\u4f26\u745e\u514b\u5927\u5b66\u3000\u526f\u6559\u6388 2001-2002 \u65b0\u4e0d\u4f26\u745e\u514b\u5927\u5b66\u3000\u6559\u6388 2002-2007 Queen&#8217;s \u5927\u5b66\u3000\u526f\u6559\u6388 (Queen\u2019s National Scholar) 2009- \u30af\u30a4\u30fc\u30f3\u30ba\u5927\u5b66\u3000\u6559\u6388 2013- \u540d\u53e4\u5c4b\u5927\u5b66\u3000Transformative\u751f\u547d\u5206\u5b50\u7814\u7a76\u6240(ITbM)\u3000\u5ba2\u5ea7\u6559\u6388\u3001\u6d77\u5916\u4e3b\u4efb\u7814\u7a76\u8005 \u517c\u4efb 2011 \u52a0\u62ff\u5927\u5316\u5b66\u4f1a\u3000\u526f\u4f1a\u957f 2012 \u52a0\u62ff\u5927\u5316\u5b66\u4f1a\u3000\u4f1a\u957f \u83b7\u5956\u7ecf\u5386 2010 NSERC Accelerator Awarde 2010 Catalysis Society Lectureship Award 2011 Clara Benson Award 2012-2013 President, Canadian Society of Chemistry 2014 Fellow, Chemical Institute of Canada 2014-2018 Scientific Council Member, The Sainsbury Lab., UK 2015-2016 Killam Research Fellow 2017 R. U. 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