{"id":3544,"date":"2015-01-10T18:51:53","date_gmt":"2015-01-10T10:51:53","guid":{"rendered":"\/\/www.gsbet888.com\/?p=3544"},"modified":"2019-08-02T18:55:56","modified_gmt":"2019-08-02T10:55:56","slug":"post-3544","status":"publish","type":"post","link":"\/\/www.gsbet888.com\/chemists\/2015\/01\/post-3544.html","title":{"rendered":"\u827e\u91cc\u4e9a\u65af\u00b7\u8a79\u59c6\u65af\u00b7\u79d1\u91cc E. J. Corey"},"content":{"rendered":"<p class=\"r\">\u827e\u91cc\u4e9a\u65af\u00b7\u8a79\u59c6\u65af\u00b7\u79d1\u91cc\uff08Elias James Corey, 1928\u5e747\u670812\u65e5\uff0d\uff09\u662f\u7f8e\u56fd\u6709\u673a\u5316\u5b66\u5bb6\u3002\u7f8e\u56fd\u54c8\u4f5b\u5927\u5b66\u6559\u6388\u30021990\u5e74\u3001\u56e0\u5728\u5f00\u53d1\u300c\u6709\u673a\u5408\u6210\u7406\u8bba\u53ca\u5176\u65b9\u6cd5\u8bba\u300d\u7b49\u7814\u7a76\u4e2d\u7684\u8d21\u732e\uff0c\u83b7\u5f97\u8bfa\u8d1d\u5c14\u5316\u5b66\u5956\u3002\u8be5\u7406\u8bba\u4f5c\u4e3a\u975e\u5e38\u590d\u6742\u7684\u5316\u5408\u7269\u5305\u62ec\u5929\u7136\u4ea7\u7269\u7684\u5408\u6210\u8def\u7ebf\u8bbe\u8ba1\u6307\u5357\u3001\u4ee5\u53ca\u9006\u5408\u6210\u5206\u6790\u624b\u6cd5\u7684\u53c2\u8003\uff0c\u79d1\u91cc\u5e74\u8fc780\u5c81\u65f6\u8fd8\u4f9d\u7136\u5168\u5fc3\u5728\u79d1\u5b66\u7814\u7a76\u4e2d\uff0c\u7edd\u5bf9\u662f\u7f8e\u56fd\u5316\u5b66\u754c\u7684\u6cf0\u6597\u7ea7\u4eba\u7269\u3002<\/p>\n<p class=\"r\">\n<h4>\u7ecf\u5386<\/h4>\n<p>1928\u5e747\u670812\u65e5\u751f\u4e8e\u9a6c\u8428\u8bf8\u585e\u5dde\u7684\u6885\u4f11\u6069\u3002<\/p>\n<p>16\u5c81\u5728Lawrence Public High School\u6bd5\u4e1a\u540e\uff0c1945\u5e74\u5728\u9ebb\u7701\u7406\u5de5(MIT)\u306b\u5165\u5b66\uff08\u5f53\u65f6Arthur C. Cope\u3001John C. Sheehan\u3001 John D. Roberts\u3001 Charles Gardner Swain\u7b49\u4e00\u4e9b\u6709\u540d\u7684\u6559\u6388\u90fd\u5728MIT\uff09\u3002<\/p>\n<p>3\u5e74\u5728MIT\u6bd5\u4e1a\u540e\uff0c\u5728Sheehan\u6559\u6388\u7ec4\u4ece\u4e8b\u76d8\u5c3c\u897f\u6797\u7684\u5408\u6210\u3001\u5728\u7ecf\u5386\u4e86\u52a9\u6559\u6388\u7684\u51e0\u5e74\u540e\uff0c\u4e8e1956\u5e74\u521a\u6ee127\u5c81\u5c31\u5df2\u7ecf\u662f\u4f0a\u5229\u8bfa\u4f0a\u5927\u5b66\u6559\u6388\u3002\u4e3b\u8981\u5728\u4e0d\u5bf9\u79f0\u5408\u6210\uff0c\u65b0\u578b\u6709\u673a\u5408\u6210\u53cd\u5e94\u7684\u5f00\u53d1\uff0c\u9176\u5316\u5b66\u7b49\u65b9\u9762\u5f00\u5c55\u7814\u7a76\u3002<\/p>\n<p>1959\u5e74\u88ab\u62db\u5165\u54c8\u4f5b\u5927\u5b66\u5316\u5b66\u79d1\u4f5c\u6559\u6388\uff0c\uff08\u5f53\u65f6\u54c8\u4f5b\u7684\u6559\u6388\u961f\u4f0d\u6709Paul D. Bartlett, Konrad Bloch, Louis F. Fieser, George B. Kistiakowski, E. G. Rochow, Frank H. Westheimer, E. B. Wilson, R. B. Woodward\uff09\u3002\u5728\u90a3\u4ee5\u540e\u3001\u6210\u529f\u5b9e\u73b0\u4e86\u8bb8\u591a\u65b0\u578b\u6709\u673a\u5408\u6210\u53cd\u5e94\u3001\u4ee5\u53ca\u590d\u6742\u5929\u7136\u4ea7\u7269\u7684\u5168\u5408\u6210\u3001\u57fa\u4e8e\u90a3\u4e9b\u57fa\u7840\u7814\u7a76\u63d0\u51fa\u4e86<b>\u9006\u5408\u6210\u5206\u6790(retrosynthesis)<\/b>\u8fd9\u4e00\u6982\u5ff5<b>\u3002\u786e\u7acb\u4e86\u590d\u6742\u6709\u673a\u5316\u5408\u7269\u5408\u6210\u7684\u8def\u7ebf\u8bbe\u8ba1\u65b9\u9488\u3002<\/b>\u4e8e1990\u5e74\u88ab\u6388\u4e88\u8bfa\u8d1d\u5c14\u5316\u5b66\u5956\u3002<\/p>\n<div>1951 \u9ebb\u7701\u7406\u5de5\u535a\u58eb\u53f7\u53d6\u5f97<br \/>\n1951 \u4f0a\u5229\u8bfa\u4f0a\u5927\u5b66(Illinois at Urbana-Champaign)\u7814\u7a76\u5458(Roger Adams, Carl S. Marvel.)<br \/>\n1956 \u4f0a\u5229\u8bfa\u4f0a\u5927\u5b66\u6559\u6388<br \/>\n1959 \u54c8\u4f5b\u5927\u5b66 \u6559\u6388<br \/>\n\u73fe\u5728 \u54c8\u4f5b\u5927\u5b66 \u540d\u8a89\u6559\u6388<\/div>\n<div><\/div>\n<div><\/div>\n<h4>\u83b7\u5956\u7ecf\u5386<\/h4>\n<div>1988 \u7f8e\u56fd\u56fd\u5bb6\u79d1\u5b66\u5956<br \/>\n1990 \u8bfa\u8d1d\u5c14\u5316\u5b66\u5956<br \/>\n2004\u00a0\u666e\u91cc\u65af\u7279\u5229\u5956\u7ae0<\/div>\n<div><\/div>\n<div><\/div>\n<h4>\u7814\u7a76<\/h4>\n<p>1990\u5e74\u56e0\u300c\u6709\u673a\u5408\u6210\u7684\u7406\u8bba\u4ee5\u53ca\u65b9\u6cd5\u8bba\u7684\u5f00\u53d1\u300d\u83b7\u8bfa\u8d1d\u5c14\u5316\u5b66\u5956\u3002\u5f00\u53d1\u4e86\u8bb8\u591a\u81f3\u4eca\u4ecd\u7136\u6709\u7528\u7684\u4eba\u540d\u53cd\u5e94\u3002\u5e94\u7528\u8fd9\u4e9b\u53cd\u5e94\u5b9e\u73b0\u4e86\u6bd4\u5982\u524d\u5217\u817a\u7d20\uff0c\u6d77\u9798\u7d20743\u7b49\u4f17\u591a\u590d\u6742\u5929\u7136\u4ea7\u7269\u7684\u5168\u5408\u6210\u3002<\/p>\n<p><strong>\u30002006\u5e74\uff0c\u4ed6\u4e0e\u4e1c\u5927\u836f\u5b66\u90e8\u67f4\u5d0e\u6559\u6388\u540c\u65f6\u62a5\u9053\u4e86\u6d41\u611f\u836f\u8fbe\u83f2\u7684\u5408\u6210\uff0c\u4e3a\u5b66\u754c\u4e00\u65f6\u8ba8\u8bba\u7684\u8bdd\u9898\u3002<\/strong>[1]\u3002<\/p>\n<p>&nbsp;<\/p>\n<h4>\u8bc4\u8bba &amp;\u5176\u4ed6<\/h4>\n<p>1. 150\u4eba\u4ee5\u4e0a\u7684\u5927\u5b66\u6559\u6388\u3001\u548c\u4f17\u591a\u5236\u836f\u516c\u53f8\u7814\u7a76\u5458\uff0c\u5728\u4e16\u754c\u4e0a\u6709\u8bb8\u591a\u5316\u5b66\u5bb6\u51fa\u4e8e\u4ed6\u7684\u95e8\u4e0b\u3002\u5728\u7f8e\u56fd\u7684\u6709\u673a\u5408\u6210\u5316\u5b66\u9886\u57df\u5927\u591a\u6570\u5316\u5b66\u5bb6\u90fd\u662f\u5206\u5c5eCorey\u6d3e\u548cEvans\u6d3e\u3002<\/p>\n<p><strong>Corey\u6d3e\u7cfb<\/strong><\/p>\n<p>\u6d77\u5916<\/p>\n<p>K.C. Nicolaou,\u00a0Michael, Chaykovsky,\u00a0Dale L. Boger, Andrew G. Myers, Phil S. Baran, David R. Liu,\u00a0 Stuart L. Schreiber, Jin Quan Yu, Philip L. Fuchs,\u00a0David Y. Gin, Dieter Seebach, Gary E. Keck,\u00a0Barry B. Snider,\u00a0Roland A. E. Winter,\u00a0Jason Kingsbury,\u00a0Edwin Vedejs,\u00a0Brian M. Stoltz,\u00a0Vinod K Singh,\u00a0David E. Cane,\u00a0Johann Mulzer,\u00a0David R. Williams,\u00a0Dieter Enders,\u00a0Wolfgang Oppolzer,\u00a0Scott A. Snyder,\u00a0Sunggak Kim,\u00a0Seiichi P.T. Matsuda<\/p>\n<p>\u65e5\u672c<\/p>\n<p>\u67f4\u5d0e\u6b63\u52dd, \u5c71\u672c\u5c1a, \u6a4b\u672c\u4fca\u4e00,\u00a0\u77f3\u539f\u4e00\u5f70, \u6ff1\u7530\u5eb7\u6b63, \u6797\u96c4\u4e8c\u90ce, \u52a0\u7d0d\u592a\u4e00,\u00a0\u6728\u8d8a\u3000\u82f1\u592b,\u00a0\u6851\u5d8b\u529f,\u00a0\u5948\u826f\u5742 \u7d18\u4e00,\u00a0\u91ce\u4f9d\u826f\u6cbb,\u00a0\u67f4\u7530 \u5d07\u5fb3,\u00a0\u8896\u5ca1 \u00a0\u5e79\u5b50,\u00a0\u7802\u585a \u654f\u660e,\u00a0\u5e02\u5ddd\u6df3\u58eb, \u9234\u6728\u6b63\u662d<\/p>\n<p>2. \u5e74\u8fc780\u5c81\u7684\u4ed6\u8fd8\u66fe\u5168\u8eab\u5fc3\u7684\u7ee7\u7eed\u79d1\u5b66\u7814\u7a76\uff0c\u771f\u7684\u8ba9\u4eba\u4e0d\u5f97\u4e0d\u4f69\u670d\u3002<\/p>\n<p>3. \u5bf9\u5f85\u7814\u7a76\u975e\u5e38\u7684\u4e25\u683c\u3001\u7814\u7a76\u5ba4\u91cc\u540c\u4e00\u8bfe\u9898\u4e4b\u95f4\u4e5f\u6709\u975e\u5e38\u6fc0\u70c8\u7684\u7ade\u4e89\u3002<\/p>\n<p>4. 2004\u5e74\u56e0Corey\u7684\u8d21\u732e\u3001\u8bbe\u7acb\u4e86\u300c<strong>Corey Award<\/strong>\u300d\u5956\uff0c2004\u5e74\u9881\u7ed9Gregory C. Fu\u30012005\u5e74\u662f David W.C. MacMillan\u30012006\u5e74\u662f Justin Du Bois\u7b49\uff0c\u8be5\u5956\u591a\u9881\u7ed9\u76f8\u5bf9\u5e74\u8f7b\u5374\u5145\u6ee1\u6d3b\u529b\u548c\u5438\u5f15\u529b\u7684\u5408\u6210\u5316\u5b66\u5bb6\u3002<\/p>\n<p>5. \u8bba\u6587\u53d1\u8868\u65f6\u7528\u7684\u7ed3\u6784\u5f0f\u975e\u5e38\u72ec\u7279\uff0c\u901a\u5e38\u5316\u5b66\u952e\u662f\u7279\u7c97\u4f53\uff0c\u5143\u7d20\u7528\u7c97\u4f53\u5b57\uff0c\u770b\u4e86\u8bba\u6587\u7684\u6458\u8981\uff0c\u5f88\u5feb\u5c31\u80fd\u7406\u89e3\u4ed6\u7684\u7814\u7a76\u5185\u5bb9\u3002<\/p>\n<p>&nbsp;<\/p>\n<h4>\u76f8\u5173\u8bba\u6587<\/h4>\n[1] Yeung, Y.-Y.; Hong, S.; Corey, E. J.\u00a0<em>J. Am. Chem. Soc.\u00a0<\/em><strong>2006<\/strong>,<em>128<\/em>, 6310. DOI:<a class=\"ext-link ext-icon-2\" title=\"\" href=\"http:\/\/dx.doi.org\/10.1021\/ja0616433\" rel=\"external\" data-wpel-target=\"_blank\">10.1021\/ja0616433<\/a><\/p>\n<p>&nbsp;<\/p>\n<p><strong>\u672c\u6587\u7248\u6743\u5c5e\u4e8e\u00a0<a href=\"\/\/www.gsbet888.com\/\">Chem-Station\u5316\u5b66\u7a7a\u95f4<\/a>\uff0c \u6b22\u8fce\u70b9\u51fb\u6309\u94ae\u5206\u4eab\uff0c\u672a\u7ecf\u8bb8\u53ef\uff0c\u8c22\u7edd\u8f6c\u8f7d\uff01<\/strong> <\/p>\n","protected":false},"excerpt":{"rendered":"\u827e\u91cc\u4e9a\u65af\u00b7\u8a79\u59c6\u65af\u00b7\u79d1\u91cc\uff08Elias James Corey, 1928\u5e747\u670812\u65e5\uff0d\uff09\u662f\u7f8e\u56fd\u6709\u673a\u5316\u5b66\u5bb6\u3002\u7f8e\u56fd\u54c8\u4f5b\u5927\u5b66\u6559\u6388\u30021990\u5e74\u3001\u56e0\u5728\u5f00\u53d1\u300c\u6709\u673a\u5408\u6210\u7406\u8bba\u53ca\u5176\u65b9\u6cd5\u8bba\u300d\u7b49\u7814\u7a76\u4e2d\u7684\u8d21\u732e\uff0c\u83b7\u5f97\u8bfa\u8d1d\u5c14\u5316\u5b66\u5956\u3002\u8be5\u7406\u8bba\u4f5c\u4e3a\u975e\u5e38\u590d\u6742\u7684\u5316\u5408\u7269\u5305\u62ec\u5929\u7136\u4ea7\u7269\u7684\u5408\u6210\u8def\u7ebf\u8bbe\u8ba1\u6307\u5357\u3001\u4ee5\u53ca\u9006\u5408\u6210\u5206\u6790\u624b\u6cd5\u7684\u53c2\u8003\uff0c\u79d1\u91cc\u5e74\u8fc780\u5c81\u65f6\u8fd8\u4f9d\u7136\u5168\u5fc3\u5728\u79d1\u5b66\u7814\u7a76\u4e2d\uff0c\u7edd\u5bf9\u662f\u7f8e\u56fd\u5316\u5b66\u754c\u7684\u6cf0\u6597\u7ea7\u4eba\u7269\u3002 \u7ecf\u5386 1928\u5e747\u670812\u65e5\u751f\u4e8e\u9a6c\u8428\u8bf8\u585e\u5dde\u7684\u6885\u4f11\u6069\u3002 16\u5c81\u5728Lawrence Public High School\u6bd5\u4e1a\u540e\uff0c1945\u5e74\u5728\u9ebb\u7701\u7406\u5de5(MIT)\u306b\u5165\u5b66\uff08\u5f53\u65f6Arthur C. Cope\u3001John C. Sheehan\u3001 John D. Roberts\u3001 Charles Gardner Swain\u7b49\u4e00\u4e9b\u6709\u540d\u7684\u6559\u6388\u90fd\u5728MIT\uff09\u3002 3\u5e74\u5728MIT\u6bd5\u4e1a\u540e\uff0c\u5728Sheehan\u6559\u6388\u7ec4\u4ece\u4e8b\u76d8\u5c3c\u897f\u6797\u7684\u5408\u6210\u3001\u5728\u7ecf\u5386\u4e86\u52a9\u6559\u6388\u7684\u51e0\u5e74\u540e\uff0c\u4e8e1956\u5e74\u521a\u6ee127\u5c81\u5c31\u5df2\u7ecf\u662f\u4f0a\u5229\u8bfa\u4f0a\u5927\u5b66\u6559\u6388\u3002\u4e3b\u8981\u5728\u4e0d\u5bf9\u79f0\u5408\u6210\uff0c\u65b0\u578b\u6709\u673a\u5408\u6210\u53cd\u5e94\u7684\u5f00\u53d1\uff0c\u9176\u5316\u5b66\u7b49\u65b9\u9762\u5f00\u5c55\u7814\u7a76\u3002 1959\u5e74\u88ab\u62db\u5165\u54c8\u4f5b\u5927\u5b66\u5316\u5b66\u79d1\u4f5c\u6559\u6388\uff0c\uff08\u5f53\u65f6\u54c8\u4f5b\u7684\u6559\u6388\u961f\u4f0d\u6709Paul D. Bartlett, Konrad Bloch, Louis F. Fieser, George B. Kistiakowski, E. G. Rochow, Frank H. Westheimer, E. B. Wilson, R. B. Woodward\uff09\u3002\u5728\u90a3\u4ee5\u540e\u3001\u6210\u529f\u5b9e\u73b0\u4e86\u8bb8\u591a\u65b0\u578b\u6709\u673a\u5408\u6210\u53cd\u5e94\u3001\u4ee5\u53ca\u590d\u6742\u5929\u7136\u4ea7\u7269\u7684\u5168\u5408\u6210\u3001\u57fa\u4e8e\u90a3\u4e9b\u57fa\u7840\u7814\u7a76\u63d0\u51fa\u4e86\u9006\u5408\u6210\u5206\u6790(retrosynthesis)\u8fd9\u4e00\u6982\u5ff5\u3002\u786e\u7acb\u4e86\u590d\u6742\u6709\u673a\u5316\u5408\u7269\u5408\u6210\u7684\u8def\u7ebf\u8bbe\u8ba1\u65b9\u9488\u3002\u4e8e1990\u5e74\u88ab\u6388\u4e88\u8bfa\u8d1d\u5c14\u5316\u5b66\u5956\u3002 1951 \u9ebb\u7701\u7406\u5de5\u535a\u58eb\u53f7\u53d6\u5f97 1951 \u4f0a\u5229\u8bfa\u4f0a\u5927\u5b66(Illinois at Urbana-Champaign)\u7814\u7a76\u5458(Roger Adams, Carl S. Marvel.) 1956 \u4f0a\u5229\u8bfa\u4f0a\u5927\u5b66\u6559\u6388 1959 \u54c8\u4f5b\u5927\u5b66 \u6559\u6388 \u73fe\u5728 \u54c8\u4f5b\u5927\u5b66 \u540d\u8a89\u6559\u6388 \u83b7\u5956\u7ecf\u5386 1988 \u7f8e\u56fd\u56fd\u5bb6\u79d1\u5b66\u5956 1990 \u8bfa\u8d1d\u5c14\u5316\u5b66\u5956 2004\u00a0\u666e\u91cc\u65af\u7279\u5229\u5956\u7ae0 \u7814\u7a76 1990\u5e74\u56e0\u300c\u6709\u673a\u5408\u6210\u7684\u7406\u8bba\u4ee5\u53ca\u65b9\u6cd5\u8bba\u7684\u5f00\u53d1\u300d\u83b7\u8bfa\u8d1d\u5c14\u5316\u5b66\u5956\u3002\u5f00\u53d1\u4e86\u8bb8\u591a\u81f3\u4eca\u4ecd\u7136\u6709\u7528\u7684\u4eba\u540d\u53cd\u5e94\u3002\u5e94\u7528\u8fd9\u4e9b\u53cd\u5e94\u5b9e\u73b0\u4e86\u6bd4\u5982\u524d\u5217\u817a\u7d20\uff0c\u6d77\u9798\u7d20743\u7b49\u4f17\u591a\u590d\u6742\u5929\u7136\u4ea7\u7269\u7684\u5168\u5408\u6210\u3002 \u30002006\u5e74\uff0c\u4ed6\u4e0e\u4e1c\u5927\u836f\u5b66\u90e8\u67f4\u5d0e\u6559\u6388\u540c\u65f6\u62a5\u9053\u4e86\u6d41\u611f\u836f\u8fbe\u83f2\u7684\u5408\u6210\uff0c\u4e3a\u5b66\u754c\u4e00\u65f6\u8ba8\u8bba\u7684\u8bdd\u9898\u3002[1]\u3002 &nbsp; \u8bc4\u8bba &amp;\u5176\u4ed6 1. 150\u4eba\u4ee5\u4e0a\u7684\u5927\u5b66\u6559\u6388\u3001\u548c\u4f17\u591a\u5236\u836f\u516c\u53f8\u7814\u7a76\u5458\uff0c\u5728\u4e16\u754c\u4e0a\u6709\u8bb8\u591a\u5316\u5b66\u5bb6\u51fa\u4e8e\u4ed6\u7684\u95e8\u4e0b\u3002\u5728\u7f8e\u56fd\u7684\u6709\u673a\u5408\u6210\u5316\u5b66\u9886\u57df\u5927\u591a\u6570\u5316\u5b66\u5bb6\u90fd\u662f\u5206\u5c5eCorey\u6d3e\u548cEvans\u6d3e\u3002 Corey\u6d3e\u7cfb \u6d77\u5916 K.C. 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