{"id":44530,"date":"2023-02-09T08:00:48","date_gmt":"2023-02-09T00:00:48","guid":{"rendered":"\/\/www.gsbet888.com\/?p=44530"},"modified":"2023-02-24T15:16:18","modified_gmt":"2023-02-24T07:16:18","slug":"%e3%80%8cspotlight-research%e3%80%8d%e5%9d%87%e7%9b%b8%e8%b6%85%e5%88%86%e5%ad%90%e8%83%b6%e5%9b%8a%e5%82%ac%e5%8c%96%e7%9a%84%e9%ab%98%e5%ba%a6%ce%b2-%e9%80%89%e6%8b%a9%e6%80%a7%e7%9a%84o-%e5%91%8b","status":"publish","type":"post","link":"\/\/www.gsbet888.com\/%e5%8c%96%e5%ad%a6%e6%9d%82%e8%ae%b0\/recentpaper\/2023\/02\/%e3%80%8cspotlight-research%e3%80%8d%e5%9d%87%e7%9b%b8%e8%b6%85%e5%88%86%e5%ad%90%e8%83%b6%e5%9b%8a%e5%82%ac%e5%8c%96%e7%9a%84%e9%ab%98%e5%ba%a6%ce%b2-%e9%80%89%e6%8b%a9%e6%80%a7%e7%9a%84o-%e5%91%8b.html","title":{"rendered":"\u300cSpotlight Research\u300d\u5747\u76f8\u8d85\u5206\u5b50\u80f6\u56ca\u50ac\u5316\u7684\u9ad8\u5ea6\u03b2-\u9009\u62e9\u6027\u7684O-\u544b\u5583\u7cd6\u82f7\u5316\u53cd\u5e94"},"content":{"rendered":"<p><strong><b>\u4f5c\u8005\uff1a\u77f3\u6cb9\u919a<\/b><\/strong><\/p>\n<p>\u672c\u671f\u70ed\u70b9\u7814\u7a76\uff0c\u6211\u4eec\u9080\u8bf7\u5230\u4e86\u672c\u6587\u7b2c\u4e00\u4f5c\u8005\uff0c\u6765\u81ea\u745e\u58eb\u5df4\u585e\u5c14\u5927\u5b66\u7684\u674e\u5929\u4efb\u535a\u58eb\u4e3a\u6211\u4eec\u5206\u4eab\u3002<\/p>\n<p>2023\u5e741\u670819\u65e5\uff0c<strong><em>J. Am. Chem. Soc<\/em><\/strong><strong><em>.<\/em><\/strong>\u5728\u7ebf\u53d1\u8868\u4e86\u6765\u81ea\u745e\u58eb\u5df4\u585e\u5c14\u5927\u5b66\u00a0Konrad Tiefenbacher \u8bfe\u9898\u7ec4\u9898\u4e3a\u300cSupramolecular Capsule-Catalyzed Highly \u03b2-Selective Furanosylation Independent of the S<sub>N<\/sub>1\/S<sub>N<\/sub>2 Reaction Pathway\u300d\u7684\u7814\u7a76\u8bba\u6587\uff1a\u91c7\u7528\u4e00\u79cd\u57fa\u4e8e\u52a8\u6001\u6c22\u952e\u7f51\u7edc\u7684\u8d85\u5206\u5b50\u80f6\u56ca\u4f5c\u4e3a\u5747\u76f8\u50ac\u5316\u5242\uff0c\u5b9e\u73b0\u4e86\u9ad8\u5ea6\u03b2-\u9009\u62e9\u6027\u7684O-\u544b\u5583\u7cd6\u82f7\u5316\u53cd\u5e94\u3002<\/p>\n<blockquote><p>\u201cSupramolecular Capsule-Catalyzed Highly \u03b2-Selective Furanosylation Independent of the S<sub>N<\/sub>1\/S<sub>N<\/sub>2 Reaction Pathway\u201d<\/p>\n<p>Tian-Ren Li, GiovanniMaria Piccini, and Konrad Tiefenbacher*<\/p>\n<p><em>J. Am. Chem. Soc.<\/em><em>\uff0c<\/em><strong>2023<\/strong><em>, <\/em>ASAP.Doi:<a href=\"https:\/\/pubs.acs.org\/doi\/10.1021\/jacs.2c13641\"><u>10.1021\/jacs.2c13641\u201d<\/u><\/a><\/p><\/blockquote>\n<h4><strong><b>Q1. <\/b><\/strong><strong><b>\u8bf7\u5bf9<\/b><\/strong>\u201cSupramolecular Capsule-Catalyzed Highly \u03b2-Selective Furanosylation Independent of the S<sub>N<\/sub>1\/S<sub>N<\/sub>2 Reaction Pathway\u201d<strong><b>\u4f5c<\/b><\/strong><strong><b>\u4e00\u4e2a\u7b80\u5355\u4ecb\u7ecd\u3002<\/b><\/strong><\/h4>\n<p>\u6211\u4eec\u91c7\u7528\u4e00\u79cd\u57fa\u4e8e\u52a8\u6001\u6c22\u952e\u7f51\u7edc\u7684\u8d85\u5206\u5b50\u80f6\u56ca\u4f5c\u4e3a\u5747\u76f8\u50ac\u5316\u5242\uff0c\u5b9e\u73b0\u4e86\u9ad8\u5ea6\u03b2-\u9009\u62e9\u6027\u7684O-\u544b\u5583\u7cd6\u82f7\u5316\u53cd\u5e94\u3002\u65e9\u4e9b\u65f6\u5019\u6211\u4eec\u66fe\u53d1\u73b0\u5728\u8be5\u8d85\u5206\u5b50\u50ac\u5316\u5242\u4e2d\u5b58\u5728\u4e00\u79cd\u88ab\u79f0\u4e3a\u2018\u8d28\u5b50\u5bfc\u7ebf\u2019\u7684\u52a8\u6001\u8d28\u5b50\u8fc1\u79fb\u8fc7\u7a0b\uff0c\u5e76\u6210\u529f\u7528\u4e8e\u9ad8\u5ea6\u03b2-\u9009\u62e9\u6027\u7684\u5421\u5583\u7cd6\u5408\u6210\u53cd\u5e94\u3002 \u5728\u6b64\u57fa\u7840\u4e0a\uff0c\u6211\u4eec\u53c8\u5bf9\u4e8e\u66f4\u5177\u6709\u6311\u6218\u6027\u7684O-\u544b\u5583\u7cd6\u82f7\u5316\u53cd\u5e94\u5728\u540c\u4e00\u50ac\u5316\u4f53\u7cfb\u4e2d\u7684\u8868\u73b0\u8fdb\u884c\u4e86\u7814\u7a76\uff0c\u9610\u660e\u4e86\u8be5\u53cd\u5e94\u7684\u673a\u7406\uff0c\u5e76\u548c\u524d\u671f\u5de5\u4f5c\u8fdb\u884c\u4e86\u5bf9\u6bd4\u3002\u7814\u7a76\u7ed3\u679c\u4ee4\u6211\u4eec\u975e\u5e38\u5174\u594b\uff0c\u6211\u4eec\u53d1\u5c55\u7684\u8fd9\u4e00\u7cfb\u5217\u8d85\u5206\u5b50\u50ac\u5316\u8fc7\u7a0b\u4e0d\u4ec5\u9002\u7528\u4e8e\u7ed3\u6784\u8fe5\u5f02\u7684\u591a\u79cd\u7cd6\u4f9b\u4f53\u7684\u03b2-\u7cd6\u82f7\u5316\u53cd\u5e94\uff0c\u5e76\u4e14\u4e0d\u53d7\u53cd\u5e94\u6210\u952e\u673a\u7406\u7684\u9650\u5236\uff0c\u4e3a\u7cd6\u5316\u5b66\u5bb6\u4eec\u7684\u5408\u6210\u5de5\u5177\u7bb1\u4e2d\u53c8\u6dfb\u52a0\u4e86\u4e00\u628a\u5f3a\u529b\u6b66\u5668\u3002<\/p>\n<h3><strong><b>Q2<\/b><\/strong><strong><b>.\u5728\u7814\u7a76\u7684\u65f6\u5019\u9047\u5230\u8fc7\u600e\u6837\u7684\u56f0\u96be\u5462\uff1f\u53c8\u662f\u600e\u6837\u514b\u670d\u7684\u5462\uff1f<\/b><\/strong><\/h3>\n<p>\u6b64\u8bfe\u9898\u7814\u7a76\u4e2d\u9047\u5230\u7684\u6700\u5927\u7684\u56f0\u96be\u53ef\u80fd\u662f\u5408\u6210\u5e94\u7528\u90e8\u5206\u3002\u6211\u4eec\u9009\u53d6\u7684\u542b\u03b2-\u6765\u82cf\u7cd6\u9aa8\u67b6\u7684\u5929\u7136\u4ea7\u7269\u5206\u5b50\u5e74\u4ee3\u6bd4\u8f83\u4e45\u8fdc\uff0c\u4e14\u4e4b\u524d\u6ca1\u6709\u88ab\u4eba\u5de5\u5408\u6210\u8fc7\uff0c\u56e0\u6b64\u53ef\u53c2\u8003\u7684\u4fe1\u606f\u5f88\u5c11\u3002\u8fd9\u7ed9\u6211\u4eec\u7684\u7ed3\u6784\u9274\u5b9a\u5de5\u4f5c\u5e26\u6765\u4e86\u5f88\u5927\u56f0\u96be\u3002\u6700\u7ec8\u662f\u91c7\u7528\u591a\u5957\u8c31\u56fe\u4ea4\u53c9\u5206\u6790\uff0c\u7ed3\u5408\u5206\u5b50\u788e\u7247\u5316\u7684\u7b56\u7565\u624d\u786e\u5b9a\u4e86\u6211\u4eec\u6240\u5f97\u5230\u7684\u5206\u5b50\u7ed3\u6784\u3002<\/p>\n<h4><strong>Q3. \u672c\u6b21\u7814\u7a76\u4e3b\u4f53\uff0c\u6709\u6ca1\u6709\u4ec0\u4e48\u8ba9\u60a8\u611f\u89c9\u7279\u522b\u8f9b\u82e6\u548c\u70e7\u8111\u5462\uff1f<\/strong><\/h4>\n<p>\u9610\u660e\u53cd\u5e94\u673a\u7406\u7684\u8fc7\u7a0b\u662f\u8fd9\u4e00\u8bfe\u9898\u6700\u4ee4\u6211\u611f\u5230\u70e7\u8111\u7684\u90e8\u5206\u3002\u56e0\u4e3a\u7cd6\u7c7b\u5206\u5b50\u7ed3\u6784\u7684\u590d\u6742\u6027\uff0c\u4ee5\u53ca\u6210\u952e\u673a\u7406\u7684\u591a\u6837\u6027\uff0c\u6539\u53d8\u4efb\u4f55\u4e00\u4e2a\u57fa\u56e2\u6216\u8005\u662f\u6539\u53d8\u67d0\u4e00\u4f4d\u70b9\u7684\u7acb\u4f53\u5316\u5b66\u4fe1\u606f\uff0c\u90fd\u4f1a\u4ee4\u53cd\u5e94\u52a8\u529b\u5b66\u53d1\u751f\u5f88\u5927\u6539\u53d8\u3002\u56e0\u6b64\u53cd\u5e94\u673a\u7406\u7684\u9610\u660e\u8fc7\u7a0b\u8017\u65f6\u5f88\u4e45\uff0c\u800c\u4e14\u76f8\u5f53\u7a0b\u5ea6\u7684\u56f0\u6270\u4e86\u6574\u4e2a\u7814\u7a76\u56e2\u961f<\/p>\n<h4><strong><b>Q4. <\/b><\/strong><strong><b>\u5c06\u6765\u60f3\u7ee7\u7eed\u7814\u7a76\u5316\u5b66\u7684\u54ea\u4e2a\u65b9\u5411\u5462\uff1f<\/b><\/strong><\/h4>\n<p>\u5c06\u6765\u5982\u679c\u6709\u673a\u4f1a\u5e0c\u671b\u80fd\u591f\u8fdb\u884c\u6709\u673a\u5316\u5b66\uff0c\u7cd6\u5316\u5b66\u4e0e\u836f\u7269\u5316\u5b66\u7ed3\u5408\u7684\u4ea4\u53c9\u5b66\u79d1\u7814\u7a76\uff0c\u671f\u671b\u80fd\u4e3a\u4eba\u7c7b\u7684\u5065\u5eb7\u548c\u533b\u836f\u53d1\u5c55\u8d21\u732e\u7ef5\u8584\u4e4b\u529b<\/p>\n<h4><strong><b>Q5. \u6700\u540e\uff0c\u6709\u4ec0\u4e48\u60f3\u5bf9\u5404\u4f4d\u8bfb\u8005\u8bf4\u7684\u5417\uff1f<\/b><\/strong><\/h4>\n<p>\u5e0c\u671b\u5404\u4f4d\u8bfb\u8005\u90fd\u80fd\u5728\u81ea\u5df1\u7684\u79d1\u7814\u5de5\u4f5c\u4e2d\u5f97\u5230\u5feb\u4e50\u548c\u81ea\u6211\u8ba4\u540c\uff0c\u6bcf\u4e00\u4e2a\u7814\u7a76\u8bfe\u9898\u90fd\u662f\u72ec\u7279\u800c\u6709\u610f\u4e49\u7684\u3002<\/p>\n<p><strong><b>\u4f5c\u8005\u6559\u80b2\u80cc\u666f\u7b80\u4ecb<\/b><\/strong><\/p>\n<p><strong><b> <img loading=\"lazy\" decoding=\"async\" class=\"aligncenter wp-image-44531 size-full\" src=\"https:\/\/assets.www.gsbet888.com\/uploads\/2023\/02\/1675869019004.png\" alt=\"\" width=\"800\" height=\"554\" srcset=\"https:\/\/assets.www.gsbet888.com\/uploads\/2023\/02\/1675869019004.png 800w, https:\/\/assets.www.gsbet888.com\/uploads\/2023\/02\/1675869019004-300x208.png 300w, https:\/\/assets.www.gsbet888.com\/uploads\/2023\/02\/1675869019004-680x471.png 680w, https:\/\/assets.www.gsbet888.com\/uploads\/2023\/02\/1675869019004-768x532.png 768w\" sizes=\"(max-width: 800px) 100vw, 800px\" \/><\/b><\/strong><\/p>\n<p><strong><b>\u6559\u80b2\u80cc\u666f\uff1a<\/b><\/strong><\/p>\n<p>2012-2018\u534e\u4e2d\u5e08\u8303\u5927\u5b66\uff0c\u535a\u58eb\u5b66\u4f4d\uff0c(\u5bfc\u5e08\uff1a\u8096\u6587\u7cbe\u6559\u6388)<\/p>\n<p>2016-2017 \u582a\u8428\u65af\u5927\u5b66\uff0c\u8054\u57f9\u535a\u58eb\uff0c(\u5bfc\u5e08\uff1aProf.\u00a0Jon Tunge)<\/p>\n<p>2018- \u00a0\u00a0\u00a0\u00a0\u00a0\u00a0\u00a0\u00a0\u5df4\u585e\u5c14\u5927\u5b66\uff0c\u535a\u58eb\u540e\uff0c(\u5bfc\u5e08\uff1aProf.\u00a0Konrad Tiefenbacher)<\/p>\n<p><strong><b>\u83b7\u5956\u7ecf\u5386\uff1a<\/b><\/strong><\/p>\n<p>\u4e2d\u56fd\u6559\u80b2\u90e8\u7814\u7a76\u751f\u56fd\u5bb6\u5956\u5b66\u91d1<\/p>\n<p>\u4e2d\u56fd\u6559\u80b2\u90e8\u535a\u58eb\u751f\u56fd\u5bb6\u5956\u5b66\u91d1<\/p>\n<p>\u535a\u96c5\u4f18\u79c0\u535a\u58eb\u751f\u5956\u5b66\u91d1<\/p>\n<p><strong><b>\u5b66\u672f\u7ecf\u5386\uff1a<\/b><\/strong><\/p>\n<p>\u81f3\u4eca\u5728\u00a0<em><i>Nature Chemistry<\/i><\/em><em><i>\u3001<\/i><\/em><em><i>\u00a0Nature Communication<\/i><\/em><em><i>\u3001<\/i><\/em><em><i>\u00a0J. Am. Chem. Soc. <\/i><\/em><em><i>\u3001<\/i><\/em><em><i>\u00a0Angewandte\u00a0Chemie International Edition <\/i><\/em><em><i>\u3001<\/i><\/em><em><i>\u00a0Chemical Society Reviews\u00a0<\/i><\/em>\u7b49\u5316\u5b66\u7c7b\u8457\u540d\u5b66\u672f\u671f\u520a\u53d1\u8868\u5b66\u672f\u8bba\u6587\u00a024 \u7bc7, \u603b\u5f15\u8d85\u8fc7\u00a01380 \u6b21\uff0c\u00a0H-index\u00a0 16\uff0c\u00a04 \u7bc7\u8bba\u6587\u88ab\u9009\u4e3a\u00a0ESI \u9ad8\u5f15\u7528\u8bba\u6587\u3002\u674e\u5929\u4efb\u535a\u58eb\u8fd8\u62c5\u4efb\u56fd\u9645\u671f\u520a Symmetry \u5ba2\u5ea7\u7f16\u8f91\u7b49\u5b66\u672f\u517c\u804c\uff0c\u540c\u65f6\u62c5\u4efb\u591a\u4e2a\u5b66\u672f\u671f\u520a\u5ba1\u7a3f\u4eba\u3002<\/p>\n<p>\u672c\u6587\u7248\u6743\u5c5e\u4e8e\u00a0Chem-Station\u5316\u5b66\u7a7a\u95f4\uff0c \u6b22\u8fce\u70b9\u51fb\u6309\u94ae\u5206\u4eab\uff0c\u672a\u7ecf\u8bb8\u53ef\uff0c\u8c22\u7edd\u8f6c\u8f7d<\/p>\n","protected":false},"excerpt":{"rendered":"\u4f5c\u8005\uff1a\u77f3\u6cb9\u919a \u672c\u671f\u70ed\u70b9\u7814\u7a76\uff0c\u6211\u4eec\u9080\u8bf7\u5230\u4e86\u672c\u6587\u7b2c\u4e00\u4f5c\u8005\uff0c\u6765\u81ea\u745e\u58eb\u5df4\u585e\u5c14\u5927\u5b66\u7684\u674e\u5929\u4efb\u535a\u58eb\u4e3a\u6211\u4eec\u5206\u4eab\u3002 2023\u5e741\u670819\u65e5\uff0cJ. Am. Chem. Soc.\u5728\u7ebf\u53d1\u8868\u4e86\u6765\u81ea\u745e\u58eb\u5df4\u585e\u5c14\u5927\u5b66\u00a0Konrad Tiefenbacher \u8bfe\u9898\u7ec4\u9898\u4e3a\u300cSupramolecular Capsule-Catalyzed Highly \u03b2-Selective Furanosylation Independent of the SN1\/SN2 Reaction Pathway\u300d\u7684\u7814\u7a76\u8bba\u6587\uff1a\u91c7\u7528\u4e00\u79cd\u57fa\u4e8e\u52a8\u6001\u6c22\u952e\u7f51\u7edc\u7684\u8d85\u5206\u5b50\u80f6\u56ca\u4f5c\u4e3a\u5747\u76f8\u50ac\u5316\u5242\uff0c\u5b9e\u73b0\u4e86\u9ad8\u5ea6\u03b2-\u9009\u62e9\u6027\u7684O-\u544b\u5583\u7cd6\u82f7\u5316\u53cd\u5e94\u3002 \u201cSupramolecular Capsule-Catalyzed Highly \u03b2-Selective Furanosylation Independent of the SN1\/SN2 Reaction Pathway\u201d Tian-Ren Li, GiovanniMaria Piccini, and Konrad Tiefenbacher* J. Am. Chem. Soc.\uff0c2023, ASAP.Doi:10.1021\/jacs.2c13641\u201d Q1. \u8bf7\u5bf9\u201cSupramolecular Capsule-Catalyzed Highly \u03b2-Selective Furanosylation Independent of the SN1\/SN2 Reaction Pathway\u201d\u4f5c\u4e00\u4e2a\u7b80\u5355\u4ecb\u7ecd\u3002 \u6211\u4eec\u91c7\u7528\u4e00\u79cd\u57fa\u4e8e\u52a8\u6001\u6c22\u952e\u7f51\u7edc\u7684\u8d85\u5206\u5b50\u80f6\u56ca\u4f5c\u4e3a\u5747\u76f8\u50ac\u5316\u5242\uff0c\u5b9e\u73b0\u4e86\u9ad8\u5ea6\u03b2-\u9009\u62e9\u6027\u7684O-\u544b\u5583\u7cd6\u82f7\u5316\u53cd\u5e94\u3002\u65e9\u4e9b\u65f6\u5019\u6211\u4eec\u66fe\u53d1\u73b0\u5728\u8be5\u8d85\u5206\u5b50\u50ac\u5316\u5242\u4e2d\u5b58\u5728\u4e00\u79cd\u88ab\u79f0\u4e3a\u2018\u8d28\u5b50\u5bfc\u7ebf\u2019\u7684\u52a8\u6001\u8d28\u5b50\u8fc1\u79fb\u8fc7\u7a0b\uff0c\u5e76\u6210\u529f\u7528\u4e8e\u9ad8\u5ea6\u03b2-\u9009\u62e9\u6027\u7684\u5421\u5583\u7cd6\u5408\u6210\u53cd\u5e94\u3002 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