{"id":46157,"date":"2023-06-16T09:25:24","date_gmt":"2023-06-16T01:25:24","guid":{"rendered":"\/\/www.gsbet888.com\/?p=46157"},"modified":"2023-06-16T09:27:16","modified_gmt":"2023-06-16T01:27:16","slug":"%e3%80%8cspotlight-research%e3%80%8d%e4%b8%8d%e5%af%b9%e7%a7%b0%e5%8a%a8%e5%8a%9b%e5%ad%a6%e6%8b%86%e5%88%86%e5%90%88%e6%88%90%e6%89%8b%e6%80%a7%ce%b1-%e7%94%b2%e7%83%af%e5%9f%ba-%ce%b3-%e4%b8%81","status":"publish","type":"post","link":"\/\/www.gsbet888.com\/%e5%8c%96%e5%ad%a6%e6%9d%82%e8%ae%b0\/recentpaper\/%e7%83%ad%e7%82%b9%e7%a0%94%e7%a9%b6\/2023\/06\/%e3%80%8cspotlight-research%e3%80%8d%e4%b8%8d%e5%af%b9%e7%a7%b0%e5%8a%a8%e5%8a%9b%e5%ad%a6%e6%8b%86%e5%88%86%e5%90%88%e6%88%90%e6%89%8b%e6%80%a7%ce%b1-%e7%94%b2%e7%83%af%e5%9f%ba-%ce%b3-%e4%b8%81.html","title":{"rendered":"\u300cSpotlight Research\u300d\u4e0d\u5bf9\u79f0\u52a8\u529b\u5b66\u62c6\u5206\u5408\u6210\u624b\u6027\u03b1-\u7532\u70ef\u57fa-\u03b3-\u4e01\u5185\u916f"},"content":{"rendered":"

\u4f5c\u8005\uff1a\u77f3\u6cb9\u919a<\/b><\/strong>\u00a0<\/b><\/strong><\/p>\n

\u672c\u671f\u70ed\u70b9\u7814\u7a76\uff0c\u6211\u4eec\u9080\u8bf7\u5230\u4e86\u672c\u6587\u7b2c\u4e00\u4f5c\u8005\u6765\u81ea\u56db\u5ddd\u5927\u5b66\u7684\u535a\u58eb\u751f\u8c2d\u653f\u4e3a\u6211\u4eec\u5206\u4eab\u3002<\/p>\n

2023\u5e746\u670811\u65e5\uff0c\u00a0<\/i><\/em>\u00a0Angew. Chem. Int. Ed<\/i><\/em>.<\/i><\/em><\/a>\u5728\u7ebf\u53d1\u8868\u4e86\u6765\u81ea\u56db\u5ddd\u5927\u5b66\u51af\u5c0f\u660e\u6559\u6388\u56e2\u961f\u9898\u4e3a\u300cAsymmetric Synthesis of \u03b1-Methylene-\u03b3-butyrolactones via Tandem Allylboration\/Lactonization: a Kinetic Resolution Process\u300d\u7684\u7814\u7a76\u8bba\u6587\u3002\u8be5\u6587\u4e2d\uff0c\u4ed6\u4eec\u5229\u7528\u624b\u6027\u53cc\u6c2e\u6c27-\u91d1\u5c5e\u914d\u5408\u7269\uff08\u51af\u50ac\u5316\u5242\uff09\u4e3a\u50ac\u5316\u5242\uff0c\u901a\u8fc7\u52a8\u529b\u5b66\u62c6\u5206\u7684\u65b9\u5f0f\uff0c\u5b9e\u73b0\u4e86\u4e0d\u5bf9\u79f0\u70ef\u4e19\u57fa\u5316\/\u5185\u916f\u5316\u4e32\u8054\u53cd\u5e94\uff0c\u5e76\u4ee5\u6b64\u5408\u6210\u4e86\u4e00\u7cfb\u5217\u03b1-\u7532\u70ef\u57fa-\u03b3-\u4e01\u5185\u916f\u7c7b\u5316\u5408\u7269\u3002<\/p>\n

\"\"<\/p>\n

\u201cAsymmetric Synthesis of \u03b1-Methylene-\u03b3-butyrolactones via Tandem Allylboration\/Lactonization: a Kinetic Resolution Process<\/strong>\u201d<\/p>\n

Zheng Tan, Long Chen, Lingyu Li, Yuzhen Li, Yao Luo, Fei Wang, Shunxi Dong*, Xiaoming Feng*<\/p>\n

Angew. Chem. Int. Ed. <\/i><\/em>2023<\/b><\/strong>, e202306146.<\/i><\/em>doi:10.1002\/anie.202306146<\/a><\/p>\n

Q1. <\/b><\/strong>\u8bf7\u5bf9\u201c<\/b><\/strong>Asymmetric Synthesis of <\/strong>\u03b1<\/strong>-Methylene-<\/strong>\u03b3<\/strong>-butyrolactones via Tandem Allylboration\/Lactonization: a Kinetic Resolution Process<\/strong>\u201d<\/b><\/strong>\u4f5c<\/b><\/strong>\u4e00\u4e2a\u7b80\u5355\u4ecb\u7ecd\u3002<\/b><\/strong><\/h4>\n

\u03b1-\u7532\u70ef\u57fa-\u03b3-\u4e01\u5185\u916f\uff08AMGBL\uff09\u9aa8\u67b6\u5e7f\u6cdb\u5b58\u5728\u4e8e\u5929\u7136\u4ea7\u7269\u548c\u836f\u7269\u5206\u5b50\u4e2d\u3002\u5f97\u76ca\u4e8e\u5176\u4f5c\u4e3a\u8fc8\u514b\u5c14\u53d7\u4f53\u9ad8\u7684\u53cd\u5e94\u6d3b\u6027\uff0c\u5b83\u4eec\u80fd\u4e0e\u4e0d\u540c\u79cd\u7c7b\u86cb\u767d\u8d28\u53d1\u751f\u5171\u8f6d\u52a0\u6210\u800c\u663e\u73b0\u51fa\u591a\u79cd\u91cd\u8981\u7684\u751f\u7269\u6d3b\u6027\u3002\u5728\u8fc7\u53bb20\u5e74\u95f4\uff0c\u5316\u5b66\u5bb6\u4eec\u53d1\u5c55\u4e86\u4e00\u7cfb\u5217\u5408\u6210AMGBL\u7c7b\u5316\u5408\u7269\u7684\u65b9\u6cd5\u3002\u5c3d\u7ba1Lewis\u9178\u50ac\u5316\uff08\u70f7\u6c27\u7fb0\u57fa\uff09\u70ef\u4e19\u57fa\u787c\u9178\u916f\u4e0e\u919b\u7684\u70ef\u4e19\u57fa\u5316\/\u5185\u916f\u5316\u53cd\u5e94\u662f\u5408\u6210\u4e0a\u8ff0\u5316\u5408\u7269\u4e00\u7c7b\u9ad8\u6548\u65b9\u6cd5\uff0c\u4f46\u8be5\u7c7b\u53cd\u5e94\u7684\u4e0d\u5bf9\u79f0\u62a5\u9053\u4e3b\u8981\u4f9d\u8d56\u4e8e\u5316\u5b66\u8ba1\u91cf\u7684\u624b\u6027\u8f85\u57fa\u3002\u8003\u8651\u5230\u5408\u6210\u6548\u7387\u4e0e\u539f\u5b50\u7ecf\u6d4e\u6027\uff0c\u5bfb\u627e\u5408\u9002\u7684\u50ac\u5316\u4f53\u7cfb\uff0c\u5b9e\u73b0\u5176\u4e0d\u5bf9\u79f0\u50ac\u5316\u5177\u6709\u91cd\u8981\u7684\u7406\u8bba\u610f\u4e49\u548c\u5e94\u7528\u524d\u666f\u3002\u57fa\u4e8e\u5bf9Lewis\u9178\u50ac\u5316\u548c\u70ef\u4e19\u57fa\u5316\/\u5185\u916f\u5316\u53cd\u5e94\u673a\u7406\u7684\u7406\u89e3\uff0c\u6211\u4eec\u5229\u7528\u8bfe\u9898\u7ec4\u539f\u521b\u7684\u624b\u6027\u53cc\u6c2e\u6c27\/\u94dd\u914d\u5408\u7269\uff08\u4e5f\u53eb\u51af\u6c0f\u50ac\u5316\u5242\uff09\u5b9e\u73b0\u4e86\u53d6\u4ee3\u70ef\u4e19\u57fa\u787c\u9178\u916f\u4e0e\u919b\u7684\u4e0d\u5bf9\u79f0\u70ef\u4e19\u57fa\u5316\/\u5185\u916f\u5316\u53cd\u5e94\u3002\u503c\u5f97\u63d0\u53ca\u7684\u662f\uff0c\u63a7\u5236\u5b9e\u9a8c\u663e\u793a\u4e0a\u8ff0\u53cd\u5e94\u624b\u6027\u63a7\u5236\u7684\u5173\u952e\u5728\u4e8e\u5bf9\u70ef\u4e19\u57fa\u5316\u4e2d\u95f4\u4f53\u7684\u4e0d\u5bf9\u79f0\u5185\u916f\u5316\u52a8\u529b\u5b66\u62c6\u5206\uff0c\u800c\u975e\u7b2c\u4e00\u6b65\u70ef\u4e19\u57fa\u5316\u3002\u9664\u624b\u6027AMGBL\u5916\uff0c\u8be5\u65b9\u6cd5\u8fd8\u80fd\u56de\u6536\u5f97\u5230\u4e00\u7cfb\u5217\u9ad8\u5149\u5b66\u7eaf\u5ea6\u7684\u9ad8\u70ef\u4e19\u9187\u7c7b\u5316\u5408\u7269\u3002\u8fd9\u4e9b\u9ad8\u70ef\u4e19\u9187\u53ef\u4ee5\u8f6c\u5316\u4e3a\u76f8\u5e94\u7684\u53cd\u6784\u578b\u53ca\u53cd\u5f0f\u7684AMGBL\u4ea7\u7269\uff0c\u5b9e\u73b0\u4e86\u5176\u7acb\u4f53\u53d1\u6563\u6027\u5408\u6210\u3002\u5229\u7528\u8fd9\u4e00\u53cd\u5e94\u4e3a\u5173\u952e\u6b65\u9aa4\uff0c\u6211\u4eec\u4e5f\u5b9e\u73b0\u4e86\u5929\u7136\u4ea7\u7269eupomatilones 2<\/b><\/strong>, 5<\/b><\/strong>, 6<\/b><\/strong>\u7684\u50ac\u5316\u4e0d\u5bf9\u79f0\u5168\u5408\u6210\u3002\u5728\u5bf9\u65b0\u5408\u6210\u7684\u624b\u6027\u4ea7\u7269\u8fdb\u884c\u4e86\u751f\u7269\u6d3b\u6027\u6d4b\u8bd5\u53d1\u73b0\u5176\u4e2d\u4e00\u4e9b\u5316\u5408\u7269\u5bf9\u4e8e\u809d\u764c\u7ec6\u80de\u5177\u6709\u8f83\u5f3a\u7684\u6291\u5236\u4f5c\u7528\uff0c\u4e14\u751f\u7269\u6d3b\u6027\u4e0e\u4ea7\u7269\u7684\u7acb\u4f53\u5316\u5b66\u6709\u5173\u3002\u6211\u4eec\u8fd8\u901a\u8fc7\u4e00\u7cfb\u5217\u63a7\u5236\u5b9e\u9a8c\uff0c\u8bc1\u660e\u4e86\u50ac\u5316\u5242\u4e3b\u8981\u4fc3\u8fdb\u4e86\u7b2c\u4e8c\u6b65\u5185\u916f\u5316\u8fc7\u7a0b\u800c\u975e\u70ef\u4e19\u57fa\u5316\uff0c\u4e0d\u5bf9\u79f0\u5185\u916f\u5316\u4e3b\u8981\u662f\u901a\u8fc7\u916f\u4ea4\u6362\u7684\u65b9\u5f0f\u800c\u975e\u78b3\u6b63\u79bb\u5b50\u9014\u5f84\u8fdb\u884c\u7684\u3002\u5728\u6b64\u57fa\u7840\u4e0a\uff0c\u6211\u4eec\u63d0\u51fa\u4e86\u53cd\u5e94\u53ef\u80fd\u7684\u53cd\u5e94\u673a\u7406\u3002<\/p>\n

\"\"<\/p>\n

Q2<\/b><\/strong>.<\/b><\/strong>\u6709\u5173\u672c\u6b21\u7814\u5728\u7814\u7a76\u7684\u65f6\u5019\u9047\u5230\u8fc7\u600e\u6837\u7684\u56f0\u96be\u5462\uff1f\u53c8\u662f\u600e\u6837\u514b\u670d\u7684\u5462\uff1f<\/b><\/strong><\/h4>\n

\u672c\u8bfe\u9898\u7684\u96be\u70b9\u4e3b\u8981\u96c6\u4e2d\u5728\u5e95\u7269\u62d3\u5c55\u3001\u884d\u751f\u548c\u673a\u7406\u5b9e\u9a8c\u4e0a\u3002\u5e78\u8fd0\u7684\u662f\u6700\u540e\u90fd\u901a\u8fc7\u4e0d\u65ad\u5730\u5c1d\u8bd5\u514b\u670d\u4e86\u3002\u5f53\u7136\u4e5f\u8fd8\u662f\u6709\u4e00\u4e9b\u95ee\u9898\u6ca1\u6709\u89e3\u51b3\uff0c\u6bd4\u5982\u5e95\u7269\u7684\u5c40\u9650\u6027\u7b49\u7b49\u3002\u6211\u89c9\u5f97\u91cd\u8981\u7684\u662f\u5fc3\u6001\u4e0a\u7684\u8c03\u6574\uff0c\u9047\u5230\u56f0\u96be\u9700\u8981\u7684\u662f\u591a\u52a0\u601d\u8003\u3001\u5c1d\u8bd5\u3001\u5206\u6790\u539f\u56e0\uff0c\u800c\u4e0d\u662f\u8ba9\u5931\u8d25\u5f71\u54cd\u81ea\u5df1\u7684\u60c5\u7eea\uff0c\u8fd9\u6837\u5373\u4fbf\u6700\u540e\u7684\u76ee\u6807\u6ca1\u6709\u8fbe\u5230\uff0c\u4e5f\u80fd\u4ece\u8fd9\u4e9b\u8fc7\u7a0b\u4e2d\u5b66\u5230\u5f88\u591a\u7ecf\u9a8c\u3002<\/p>\n

Q<\/strong>3.<\/strong>\u00a0<\/strong>\u672c\u6b21\u7814\u7a76\u4e3b\u4f53\uff0c\u6709\u6ca1\u6709\u4ec0\u4e48\u8ba9\u60a8\u611f\u89c9\u7279\u522b\u8f9b\u82e6\u548c\u70e7\u8111\u5462\uff1f<\/strong><\/h4>\n

\u5728\u6269\u5c55\u5e95\u7269\u7684\u8fc7\u7a0b\u4e2d\u9047\u5230\u4e86\u5f88\u591a\u96be\u9898\uff0c\u5408\u6210\u4e86\u5f88\u591a\u7684\u70ef\u4e19\u57fa\u5e95\u7269\uff0c\u4f46\u662f\u8fd9\u4e9b\u5e95\u7269\u5728\u6211\u7684\u6700\u4f18\u6761\u4ef6\u4e0b\u5747\u6ca1\u6709\u5f97\u5230\u597d\u7684\u7ed3\u679c\uff0c\u540c\u65f6\u4ea7\u7269\u7684\u5206\u79bb\u7eaf\u5316\u4e5f\u8017\u8d39\u4e86\u5f88\u5927\u7684\u7cbe\u529b\u3002<\/p>\n

Q<\/b><\/strong>4.<\/b><\/strong>\u00a0<\/b><\/strong>\u5c06\u6765\u60f3\u7ee7\u7eed\u7814\u7a76\u5316\u5b66\u7684\u54ea\u4e2a\u65b9\u5411\u5462\uff1f<\/b><\/strong><\/h4>\n

\u672a\u6765\u8fd8\u662f\u60f3\u7ee7\u7eed\u4e0d\u5bf9\u79f0\u70ef\u4e19\u57fa\u5316\u53cd\u5e94\u9886\u57df\u7684\u7814\u7a76\uff0c\u70ef\u4e19\u57fa\u5316\u53cd\u5e94\u8fd8\u6709\u8bb8\u591a\u53ef\u4ee5\u63a2\u7d22\u7684\u5730\u65b9\u3002<\/p>\n

Q<\/b><\/strong>5.<\/b><\/strong>\u00a0<\/b><\/strong>\u6700\u540e\uff0c\u6709\u4ec0\u4e48\u60f3\u5bf9\u5404\u4f4d\u8bfb\u8005\u8bf4\u7684\u5417\uff1f<\/b><\/strong><\/p>\n

\u5e0c\u671b\u5728\u505a\u79d1\u5b66\u7814\u7a76\u7684\u5404\u4f4d\u90fd\u80fd\u627e\u5230\u81ea\u5df1\u611f\u5174\u8da3\u7684\u7814\u7a76\u65b9\u5411\uff0c\u597d\u5947\u5fc3\u6c38\u8fdc\u662f\u79d1\u7814\u6700\u5927\u7684\u52a8\u529b\uff0c\u65e0\u8bba\u6700\u540e\u8bba\u6587\u53d1\u8868\u5982\u4f55\uff0c\u6700\u91cd\u8981\u7684\u662f\u89e3\u51b3\u79d1\u5b66\u95ee\u9898\uff0c\u63a2\u7d22\u672a\u77e5\uff0c\u4eab\u53d7\u79d1\u7814\u8fc7\u7a0b\u4e2d\u7684\u4e50\u8da3\u3002<\/p>\n

\u4f5c\u8005\u6559\u80b2\u80cc\u666f\u7b80\u4ecb<\/b><\/strong><\/h4>\n

\"\"<\/p>\n

\u6559\u80b2\u80cc\u666f\uff1a<\/b><\/strong><\/p>\n

2015-2019\uff0c \u56db\u5ddd\u5927\u5b66\uff0c \u672c\u79d1<\/p>\n

2019-2021\uff0c \u56db\u5ddd\u5927\u5b66\uff0c \u7855\u58eb<\/p>\n

2021-2023\uff0c \u56db\u5ddd\u5927\u5b66\uff0c\u535a\u58eb<\/p>\n

\u672c\u6587\u7248\u6743\u5c5e\u4e8e\u00a0Chem-Station\u5316\u5b66\u7a7a\u95f4\uff0c \u6b22\u8fce\u70b9\u51fb\u6309\u94ae\u5206\u4eab\uff0c\u672a\u7ecf\u8bb8\u53ef\uff0c\u8c22\u7edd\u8f6c\u8f7d<\/p>\n","protected":false},"excerpt":{"rendered":"\u4f5c\u8005\uff1a\u77f3\u6cb9\u919a\u00a0 \u672c\u671f\u70ed\u70b9\u7814\u7a76\uff0c\u6211\u4eec\u9080\u8bf7\u5230\u4e86\u672c\u6587\u7b2c\u4e00\u4f5c\u8005\u6765\u81ea\u56db\u5ddd\u5927\u5b66\u7684\u535a\u58eb\u751f\u8c2d\u653f\u4e3a\u6211\u4eec\u5206\u4eab\u3002 2023\u5e746\u670811\u65e5\uff0c\u00a0\u00a0Angew. Chem. Int. Ed.\u5728\u7ebf\u53d1\u8868\u4e86\u6765\u81ea\u56db\u5ddd\u5927\u5b66\u51af\u5c0f\u660e\u6559\u6388\u56e2\u961f\u9898\u4e3a\u300cAsymmetric Synthesis of \u03b1-Methylene-\u03b3-butyrolactones via Tandem Allylboration\/Lactonization: a Kinetic Resolution Process\u300d\u7684\u7814\u7a76\u8bba\u6587\u3002\u8be5\u6587\u4e2d\uff0c\u4ed6\u4eec\u5229\u7528\u624b\u6027\u53cc\u6c2e\u6c27-\u91d1\u5c5e\u914d\u5408\u7269\uff08\u51af\u50ac\u5316\u5242\uff09\u4e3a\u50ac\u5316\u5242\uff0c\u901a\u8fc7\u52a8\u529b\u5b66\u62c6\u5206\u7684\u65b9\u5f0f\uff0c\u5b9e\u73b0\u4e86\u4e0d\u5bf9\u79f0\u70ef\u4e19\u57fa\u5316\/\u5185\u916f\u5316\u4e32\u8054\u53cd\u5e94\uff0c\u5e76\u4ee5\u6b64\u5408\u6210\u4e86\u4e00\u7cfb\u5217\u03b1-\u7532\u70ef\u57fa-\u03b3-\u4e01\u5185\u916f\u7c7b\u5316\u5408\u7269\u3002 \u201cAsymmetric Synthesis of \u03b1-Methylene-\u03b3-butyrolactones via Tandem Allylboration\/Lactonization: a Kinetic Resolution Process\u201d Zheng Tan, Long Chen, Lingyu Li, Yuzhen Li, Yao Luo, Fei Wang, Shunxi Dong*, Xiaoming Feng* Angew. Chem. Int. Ed. 2023, e202306146.doi:10.1002\/anie.202306146 Q1. \u8bf7\u5bf9\u201cAsymmetric Synthesis of \u03b1-Methylene-\u03b3-butyrolactones via Tandem Allylboration\/Lactonization: a Kinetic Resolution Process\u201d\u4f5c\u4e00\u4e2a\u7b80\u5355\u4ecb\u7ecd\u3002 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